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During the suspension, Ajax were in contact with other European clubs interested in Suárez.
On 28 January 2011, they accepted a €26.5 million (£22.8 million) offer for Suárez from Premier League club Liverpool.
In his first season at Barcelona, Suárez starred in an attacking trio alongside Lionel Messi and Neymar, helping the club win a historic second continental treble of La Liga, the Copa del Rey and the UEFA Champions League.
The trio scored a total of 122 goals that season, the most for an attacking front three in Spanish football history.
On 20 November 2010, Suárez bit PSV's Otman Bakkal on the shoulder during a 0–0 draw.
A year later, he helped Ajax secure the Eredivisie title, and scored his 100th Ajax goal.
In his second season at the club, Suárez won his first Pichichi Trophy as well as his second European Golden Shoe, for which, he became the first player since 2009 to win both awards other than Messi or Ronaldo. At the 2010 FIFA World Cup, he played an important role in Uruguay's fourth-place finish, scoring three goals, as well as controversially blocking a goal-bound extra time header with his hands during the quarter-final against Ghana.